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Temperature-controlled metal/ligand stoichiometric ratio in Ag-TCNE coordination networks.

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The deposition of tetracyanoethylene (TCNE) on Ag(111), both at Room Temperature (RT, 300K) and low temperatures (150 K), leads to the formation of coordination networks involving silver adatoms, as revealed by Variable-Temperature Scanning Tunneling Microscopy (VT-STM). Our results indicate that TCNE molecules etch away material from the step edges and possibly also from the terraces, which facilitates the formation of the observed coordination networks. Moreover, such process is temperature...

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